Studies towards the total synthesis of narbonolide: stereoselective preparation of the C1–C10 fragment
2008
Abstract An efficient stereoselective synthesis of the C1–C10 fragment of narbonolide is reported. The stereocentres at C2, 3, 4, 5, 8 and 9 in fragment 5 can be generated via an iterative asymmetric acyl-thiazolidinethione aldol reaction, whereas the stereocentre at C6 is installed by means of Myers alkylation.
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