The surface of topological insulators is proposed as a promising platform for spintronics and quantum information applications. In particular, when time- reversal symmetry is broken, topological surface states are expected to exhibit a wide range of exotic spin phenomena for potential implementation in electronics. Such devices need to be fabricated using nanoscale artificial thin films. It is of critical importance to study the spin behavior of artificial topological MBE thin films associated with magnetic dopants, and with regards to quantum size effects related to surface-to-surface tunneling as well as experimentally isolate time-reversal breaking from non-intrinsic surface electronic gaps. Here we present observation of the first (and thorough) study of magnetically induced spin reorientation phenomena on the surface of a topological insulator. Our results reveal dramatic rearrangements of the spin configuration upon magnetic doping contrasted with chemically similar nonmagnetic doping as well as with quantum tunneling phenomena in ultra-thin high quality MBE films. While we observe that the spin rearrangement induced by quantum tunneling occurs in a time-reversal invariant fashion, we present critical and systematic observation of an out-of-plane spin texture evolution correlated with magnetic interactions, which breaks time-reversal symmetry, demonstrating microscopic TRB at a Kramers' point on the surface.
We present angle-resolved photoemission studies on the rare-earth hexaboride YbB$_6$, which has recently been predicted to be a topological Kondo insulator. Our data do not agree with the prediction and instead show that YbB$_6$ exhibits a novel topological insulator state in the absence of a Kondo mechanism. We find that the Fermi level electronic structure of YbB$_6$ has three 2D Dirac cone like surface states enclosing the Kramers' points, while the f-orbital which would be relevant for the Kondo mechanism is $\sim1$ eV below the Fermi level. Our first-principles calculation shows that the topological state which we observe in YbB$_6$ is due to an inversion between Yb $d$ and B $p$ bands. These experimental and theoretical results provide a new approach for realizing novel correlated topological insulator states in rare-earth materials.
Spin polarization effects in nonmagnetic materials are generally believed as an outcome of spin-orbit coupling provided that the global inversion symmetry is lacking, also known as 'spin-momentum locking'. The recently discovered hidden spin polarization indicates that specific atomic site asymmetry could also induce measurable spin polarization, leading to a paradigm shift to centrosymmetric crystals for potential spintronic applications. Here, combining spin- and angle-resolved photoemission spectroscopy and theoretical calculations, we report distinct spin-layer locking phenomena surrounding different high-symmetry momenta in a centrosymmetric, layered material BiOI. The measured spin is highly polarized along the Brillouin zone boundary, while is almost vanishing around the zone center due to its nonsymmorphic crystal structure. Our work not only demonstrates the existence of hidden spin polarization, but also uncovers the microscopic mechanism of the way spin, momentum and layer locking to each other, shedding lights on the design metrics for future spintronic devices.
We review recent progress in the electronic structure study of intrinsic magnetic topological insulators (MnBi$_2$Te$_4$)(Bi$_2$Te$_3$)$_n$ ($n=0,1,2,3$) family. Specifically, we focus on the ubiquitously (nearly) gapless behavior of the topological surface state Dirac cone observed by photoemission spectroscopy, even though a large Dirac gap is expected because of surface ferromagnetic order. The dichotomy between experiment and theory concerning this gap behavior is perhaps the most critical and puzzling question in this frontier. We discuss various proposals accounting for the lack of magnetic effect on the topological surface state Dirac cone, which are mainly categorized into two pictures, magnetic reconfiguration, and topological surface state redistribution. Band engineering towards opening a magnetic gap of topological surface states provides great opportunities to realize quantized topological transport and axion electrodynamics at higher temperatures.
Mn[Formula: see text]Ir/CoFe bilayer is a prototypical exchange-coupled antiferromagnet (AF)-ferromagnet (FM) system. Nevertheless, a strong exchange coupling between FM and rare-earth(RE) interfaces of Fe/Dy and Fe/Tb has been established earlier. Strong coupling at the FM-RE interface originates from the number of irreversible spins owing to the imbalance in the non-collinear configuration in RE. However, exchange coupling between AF-RE could not be established due to the minimal number of irreversible spins in AF and RE. A frustrated inter-domain magnetic interaction leads to the coexistence of spin-freezing-like ordering around the temperature range of helical spin modulation at the exchange-coupled interfaces of RE-based specimens. To overcome the lack of coupling between the AF-RE interface, we use a sandwich structure of AF-FM-RE layers (Mn[Formula: see text]Ir/CoFe/Dy) as we demonstrate establishing considerable exchange bias in the system. Changing the bias direction during field cooling introduces possible differences in non-collinear directions (helicities), which affects the number of irreversible spins and consequent exchange coupling differently for opposite directions. The non-collinear structures in RE are topologically stable; thus, their directions of orientation can be regarded as an additional degree of freedom, which can be manipulated in all-spin-based technology.
Centimeter-size KBBF and RBBF single crystals have been grown hydrothermally for NLO applications. Second harmonic generation of 800 nm fundamental light has been demonstrated using both KBBF and RBBF in preliminary studies.
Recently, a crystalline-symmetry-protected three-dimensional (3D) bulk Dirac semimetal phase has been experimentally identified in a stoichiometric high-mobility compound, ${\mathrm{Cd}}_{3}{\mathrm{As}}_{2}$. The Dirac state observed in ${\mathrm{Cd}}_{3}{\mathrm{As}}_{2}$ has been attributed to originate mostly from the bulk state while calculations show that the bulk and surface states overlap over the entire Dirac dispersion energy range. In this study we unambiguously reveal doping induced evolution of the ground state of surface and bulk electron dynamics in a 3D Dirac semimetal. The technique demonstrated in this study by simultaneously using angle-resolved photoemission spectroscopy (ARPES) and in situ surface deposition isolates the surface and bulk states in ${\mathrm{Cd}}_{3}{\mathrm{As}}_{2}$. Our experimental results provide a method for tuning the chemical potential as well as to observe surface states degenerate with bulk states, which will be useful for future applications of a 3D Dirac semimetal.
In the past decade, magnetic topological insulators have been an important focus in condensed matter physics research. The intricate interplay between the nontrivial band topology and spin, orbit, charge, and dimensionality degrees of freedom can give rise to abundant exotic topological quantum states and topological phase transitions. Measuring the transport properties of magnetic topological insulators is a crucial approach to exploring their exotic properties, which is of significant scientific importance in deepening our understanding of topological quantum states. Simultaneously, it also holds substantial potential applications in the development of novel low-power electronic devices. In this work, experimental progress of transport researches of magnetic topological insulators is reviewed, including quantum anomalous Hall effect and topological quantum phase transitions in magnetically doped topological insulators, the quantum anomalous Hall phase, axion insulator phase and Chern insulator phase in intrinsic antiferromagnetic topological insulator MnBi<sub>2</sub>Te<sub>4</sub>, as well as the helical phase emerged from the Chern insulator in pulsed high magnetic fields. Finally, this work analyzes the future direction of development in magnetic topological insulators, and the transport phenomena that have not been understood in these systems, offering an insight into and perspectives on the potential breakthroughs to be achieved in this area of research.
A perpetual quest in the field of topological quantum matter is to search for electronic phases with unprecedented band topology and transport phenomena. The most prominent example is the discovery of topological insulators, in which band inversion leads to topologically nontrivial bulk electronic structure and metallic boundary states. In two-dimensional topological insulators with time-reversal symmetry, a pair of helical edge states gives rise to the quantum spin Hall effect. When the time-reversal symmetry is broken by magnetic order, only one chiral edge mode remains and the quantum anomalous Hall effect emerges in zero magnetic field. This quantum Hall phase without Landau levels, first observed in magnetically doped topological insulators, is now called the Chern insulator. The recently discovered MnBi2Te4 combines intrinsic magnetism and nontrivial topology in one material, providing an ideal platform for exploring novel topological phases. Here, we investigate the transport properties of exfoliated MnBi2Te4 in exceedingly high magnetic fields up to 60 T. By varying the gate voltage, we observe systematic and yet uniquely complex evolution of quantized Hall plateaus with Chern numbers from C = -3 to +2. More surprisingly, a novel phase characterized by an extremely broad zero Hall plateau emerges as the most robust ground state in the high field limit. Theoretical calculations reveal that this C = 0 phase arises from the coexistence of a connate Chern band with C = -1 and a Zeeman-effect-induced Chern band with C = +1, as corroborated by nonlocal transport measurements. This helical Chern insulator phase with broken time-reversal symmetry represents an unexpected new member of the quantum Hall family, and manifests a new route to change the band topology by using magnetic field.
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