An Liao

East China University of Technology

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Chunhui Dai

East China University of Technology

Xuezhong Gong

Qingdao University

Zhaocen Dong

Qingdao University

Yachao Zhang

East China University of Technology

Chao Zeng

Jiangxi Normal University

Qing Liu

East China University of Technology

Wei Wu

East China University of Technology

Waner Li

East China University of Technology

Zhixin Zhou

East China University of Technology

Mantao Chen

East China University of Technology

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East China University of Technology

University of Michigan–Ann Arbor

Ann Arbor Center for Independent Living

Nanjing University

Qingdao University

City University of Hong Kong

Laboratoire d'Informatique de Paris-Nord

Michigan United

National University of Singapore

Massachusetts Institute of Technology

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Metal–Salen‐Incorporated conjugated microporous polymers as robust artificial leaves for solar‐driven reduction of atmospheric CO₂ with H₂O

Carbon Energy (2024)

Wei Wu Zhaocen Dong Mantao Chen Waner Li An Liao

Abstract Exploration of efficient and stable photocatalysts to mimic natural leaves for the conversion of atmospheric CO 2 into hydrocarbons utilizing solar light is very important but remains a major challenge. Herein, we report the design of four novel metal–salen‐incorporated conjugated microporous polymers as robust artificial leaves for photoreduction of atmospheric CO 2 with gaseous water. Owing to the rich nitrogen and oxygen moieties in the polymeric frameworks, they show a maximum CO 2 adsorption capacity of 46.1 cm 3 g −1 and adsorption selectivity for CO 2 /N 2 of up to 82 at 273 K. Under air atmosphere and simulated solar light (100 mW cm −2 ), TEPT‐Zn shows an excellent CO yield of 304.96 μmol h −1 g −1 with a selectivity of approximately 100%, which represents one of the best results in terms of organic photocatalysts for gas‐phase CO 2 photoreduction so far. Furthermore, only small degradation in the CO yield is observed even after 120‐h continuous illumination. More importantly, a good CO yield of 152.52 μmol g −1 was achieved by directly exposing the photocatalytic reaction of TEPT‐Zn in an outdoor environment for 3 h (25–28°C, 52.3 ± 7.9 mW cm −2 ). This work provides an avenue for the continued development of advanced polymers toward gas‐phase photoconversion of CO 2 from air.

Conjugated microporous polymer

10.1002/cey2.646

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Cover Image, Volume 7, Number 1, January 2025

Carbon Energy (2025)

Wei Wu Zhaocen Dong Mantao Chen Waner Li An Liao

10.1002/cey2.722

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Acute Dietary Restriction Acts via TOR, PP2A, and Myc Signaling to Boost Innate Immunity in Drosophila

Cell Reports (2017)

Jung-Eun Lee Morsi S Rayyan An Liao Isaac Edery Scott D. Pletcher

Dietary restriction promotes health and longevity across taxa through mechanisms that are largely unknown. Here, we show that acute yeast restriction significantly improves the ability of adult female Drosophila melanogaster to resist pathogenic bacterial infections through an immune pathway involving downregulation of target of rapamycin (TOR) signaling, which stabilizes the transcription factor Myc by increasing the steady-state level of its phosphorylated forms through decreased activity of protein phosphatase 2A. Upregulation of Myc through genetic and pharmacological means mimicked the effects of yeast restriction in fully fed flies, identifying Myc as a pro-immune molecule. Short-term dietary or pharmacological interventions that modulate TOR-PP2A-Myc signaling may provide an effective method to enhance immunity in vulnerable human populations.

TOR signaling

10.1016/j.celrep.2017.06.052

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Effect of relative humidity and pre-annealing temperature on spin-coated zinc tin oxide films made via the metal–organic decomposition route

Journal of Materials Chemistry C (2017)

Youngbae Son An Liao Rebecca L. Peterson

Solution-processed zinc tin oxide thin-film transistor using metal–organic decomposition achieves wide process window in terms of ambient humidity during deposition.

Tin oxide

Spin Coating

10.1039/c7tc02343j

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Citations (18)