We present protocols relying on coherent rotations and squeezing for the creation of arbitrary symmetric states. The obtained states can be further transferred to traveling photonic states via spontaneous emission, enabling engineered quantum light states.
Collective optical properties can emerge from an ordered ensemble of emitters due to interactions between the individual units. Superlattices of halide perovskite nanocrystals exhibit collective light emission, influenced by dipole–dipole interactions between simultaneously excited nanocrystals. This coupling changes both the emission energy and rate compared to the emission of uncoupled nanocrystals. We demonstrate how quantum confinement governs the nature of the coupling between the nanocrystals in the ensemble. The extent of confinement is modified by controlling the nanocrystal size or by compositional control over the Bohr radius. In superlattices made of weakly confined nanocrystals, the collective emission is red-shifted with a faster emission rate, showing the key characteristics of superfluorescence. In contrast, the collective emission of stronger quantum-confined nanocrystals is blue-shifted with a slower emission rate. Both types of collective emission exhibit correlative multiphoton emission bursts, showing distinct photon bunching emission statistics. The quantum confinement changes the preferred alignment of transition dipoles within the nanocrystal and switches the relative dipole orientation between neighbors, resulting in opposite collective optical behaviors. Our results extend these collective effects to relatively high temperatures and provide a better understanding of exciton interactions and collective emission phenomena at the solid state.
For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high harmonics. We derive a formula for the quantum state of the high harmonics, when driven by arbitrary quantum light states, and then explore specific cases of experimental relevance. Specifically, for a moderately squeezed pump, HHG driven by squeezed coherent light results in squeezed high harmonics. Harmonic squeezing is optimized by syncing ionization times with the pump's squeezing phase. Beyond this regime, as pump squeezing is increased, the harmonics initially acquire squeezed thermal photon statistics, and then occupy an intricate quantum state which strongly depends on the semi-classical nonlinear response function of the interacting system. Our results pave the way for the generation of squeezed extreme-ultraviolet ultrashort pulses, and, more generally, quantum frequency conversion into previously inaccessible spectral ranges, which may enable ultrasensitive attosecond metrology.
The ultrafast dynamics of charge carriers in solids plays a pivotal role in emerging optoelectronics, photonics, energy harvesting, and quantum technology applications. However, the investigation and direct visualization of such non-equilibrium transport phenomena remains as a long-standing challenge, owing to the nanometer-femtosecond spatio-temporal scales at which the charge carriers evolve. Here, we propose and demonstrate a novel interaction mechanism enabling nanoscale imaging of the femtosecond dynamics of charge carriers in solids. This imaging modality, which we name charge dynamics electron microscopy (CDEM), exploits the strong interaction between terahertz (THz) electromagnetic near fields produced by the moving charges and synchronized free-electron pulses in an ultrafast scanning transmission electron microscope. The measured free-electron energy at different spatio-temporal coordinates allows us to directly retrieve the THz near-field amplitude and phase, from which we reconstruct movies of the generated charges by comparison with microscopic theory. The introduced CDEM technique thus allows us to investigate previously inaccessible spatio-temporal regimes of charge dynamics in solids, for example revealing new insight into the photo-Dember effect, showing oscillations of photo-generated electron-hole distributions inside a semiconductor. Our work lays the foundation for exploring a wide range of previously inaccessible charge-transport phenomena in condensed matter using ultrafast electron microscopy.
We present a method to produce entangled photon pairs in the extreme ultraviolet (EUV) and X-ray regime, using a new highly nonperturbative nonlinear optical process which we term “high harmonic down conversion” (HHDC).
The manipulation of quantum many-body systems is a crucial goal in quantum science. Entangled quantum states that are symmetric under qubits permutation are of growing interest. Yet, the creation and control of symmetric states has remained a challenge. Here, we introduce a method to universally control symmetric states, proposing a scheme that relies solely on coherent rotations and spin squeezing. We present protocols for the creation of different symmetric states including Schr\"odinger's cat and Gottesman-Kitaev-Preskill states. The obtained symmetric states can be transferred to traveling photonic states via spontaneous emission, providing a powerful approach for engineering desired quantum photonic states.
We show how modulated free-electron wavepackets can extract the ultrafast dynamics of arbitrary quantum light states in nanophotonic resonators and waveguides, capturing decoherence and other interactions.
Parametric x-ray radiation (PXR) is a prospective mechanism for producing directional, tunable, and quasi-coherent x-rays in laboratory-scale dimensions, yet it is limited by heat dissipation and self-absorption. Resolving these limits, we show the PXR source flux is suitable for medical imaging and x-ray spectroscopy. We discuss the experimental feasibility of these findings for a compact commercial PXR source.
Compact laboratory-scale X-ray sources still rely on the same fundamental principles as in the first X-ray tubes developed more than a century ago. In recent years, significant research and development have focused on large-scale X-ray sources such as synchrotrons and free-electron lasers, leading to the generation of high-brightness coherent X-rays. However, the large size and high costs of such sources prevent their widespread use. The quest for a compact and coherent Xray source has long been a critical objective in modern physics, gaining further importance in recent years for industrial applications and fundamental scientific research. Here, we review the physical mechanisms governing compact coherent X-ray generation. Of current interest are coherent periodic interactions of free electrons in crystalline materials, creating hard X-rays via a mechanism known as parametric X-ray radiation (PXR). Over the past decade, X-ray sources leveraging this mechanism have demonstrated state-of-the-art tunability, directionality, and broad spatial coherence, enabling X-ray phase-contrast imaging on a compact scale. The coming years are expected to show substantial miniaturization of compact X-ray sources, facilitated by progress in electron beam technologies. This review compares the most promising mechanisms used for hard-X-ray generation, contrasting parametric X-ray radiation with inverse Compton scattering and characteristic radiation from a liquid-jet anode. We cover the most recent advancements, including the development of new materials, innovative geometrical designs, and specialized optimization techniques, aiming toward X-ray flux levels suitable for medical imaging and X-ray spectroscopy in compact scales.
We find that high harmonic generation strongly depends on the photon statistics of the driving field. Specifically, squeezed light exhibits a strongly extended cutoff relative to classical light, creating high harmonics at far greater efficiency.
'/%3e%3cuse xlink:href='%23a' transform='translate(288.889 -214.211)'/%3e%3cuse xlink:href='%23a' transform='translate(108 342.749)'/%3e%3cuse xlink:href='%23a' transform='translate(469.189 342.749)'/%3e%3c/svg%3e)
