Cong‐Ying Zhou

Jinan University

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Chi‐Ming Che

University of Hong Kong

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Zhen Guo

Tsinghua University

Haixu Wang

Anshan Normal University

Jinhu Wei

South China University of Technology

Jie‐Sheng Huang

Wuhan University

Zhen Guo

Kam‐Hung Low

State Key Laboratory of Synthetic Chemistry

Chun‐Wai Tse

State Key Laboratory of Synthetic Chemistry

Qingyun Wan

State Key Laboratory of Synthetic Chemistry

Wing‐Yiu Yu

Hong Kong Polytechnic University

Cooperative Institutions

University of Hong Kong

State Key Laboratory of Synthetic Chemistry

Chinese Academy of Sciences

Jinan University

Taiyuan University of Technology

Peking University

Sun Yat-sen University

University of Chinese Academy of Sciences

Hong Kong Polytechnic University

Shanghai Institute of Organic Chemistry

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Highly stable Ni₈-pyrazolate metal–organic frameworks for adsorption of methylene blue from water

New Journal of Chemistry (2023)

Guoqiang Wu Kun Wu Ying Wang Jie Luo Cong‐Ying Zhou

Metallosalen-based Ni 8 -pyrazolate metal–organic frameworks were prepared, and they exhibited exceptional chemical stability and high efficiency in the removal of methylene blue (MB) from water.

Methylene blue

Methylene

10.1039/d3nj03052k

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Citations (2)

Divergent Construction of Heterocycles by SOMOphilic Isocyanide Insertion under N-Heterocyclic Carbene Catalysis

Organic Letters (2022)

Qianrong Li Cong‐Ying Zhou Chengming Wang

A variety of phenanthridines are rapidly constructed by an N-heterocyclic carbene (NHC)-catalyzed SOMOphilic isocyanide insertion-initiated homolytic aromatic substitution-type radical cyclization in the absence of any light, transition metals, and external oxidants. The aldehyde-free, scalable, and operationally simple protocol tolerates diverse functionalized biaryl isonitriles and activated α-halides. Moreover, it can be further applied to the divergent construction of other N-heterocycles. Preliminary mechanistic studies disclose that an NHC-derived radical cation intermediate is possibly involved.

Homolysis

Divergent synthesis

10.1021/acs.orglett.2c03148

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Citations (16)

Ruthenium(II) Porphyrin Catalyzed Tandem Carbonyl Ylide Formation and 1,3‐Dipolar Cycloaddition Reactions of α‐Diazo Ketones.

ChemInform (2003)

Cong‐Ying Zhou Wing‐Yiu Yu Chi‐Ming Che

Abstract For Abstract see ChemInform Abstract in Full Text.

Ylide

Tandem

10.1002/chin.200304039

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Cobalt(II) Porphyrin‐Catalyzed Intramolecular Cyclopropanation of N‐Alkyl Indoles/Pyrroles with Alkylcarbene: Efficient Synthesis of Polycyclic N‐Heterocycles

Angewandte Chemie (2015)

Rajasekar Reddy Annapureddy Fei Hao Kai Wu Cong‐Ying Zhou Chi‐Ming Che

Abstract A protocol on chemoselective cobalt(II) porphyrin‐catalyzed intramolecular cyclopropanation of N‐alkyl indoles/pyrroles with alkylcarbenes has been developed. The reaction enables the rapid construction of a range of nitrogen‐containing polycyclic compounds in moderate to high yields from readily accessible materials. These N‐containing polycyclic compounds can be converted into a variety of N‐heterocycles with potential synthetic and biological interest. Compared to their N‐tosylhydrazone counterparts, the use of bulky N‐2,4,6‐triisopropylbenzenesulfonyl hydrazones as carbene precursors allows cyclopropanation to occur under milder reaction conditions.

10.1002/ange.201506418

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Citations (8)

CCDC 1890161: Experimental Crystal Structure Determination

The Cambridge Structural Database (2021)

Haixu Wang Qingyun Wan Kai Wu Kam‐Hung Low Chen Yang

10.5517/ccdc.csd.cc21fvy9

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Rhodium-Catalyzed C(sp²)–O Cross Couplings of Diazo Quinones with Phenols to Construct Diaryl Ethers

Organic Letters (2023)

Fu Zhen XiaoKun Wang Xiaoyu Ren Zhen Guo Chengming Wang

The diaryl ether represents a prevalent structural motif found in numerous biologically active molecules. Herein, we describe a dirhodium-catalyzed C(sp

Coupling reaction

10.1021/acs.orglett.3c03969

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Citations (3)

ChemInform Abstract: Highly Efficient Oxidative Carbon—Carbon Coupling with SBA‐15‐Support Iron Terpyridine Catalyst.

ChemInform (2010)

Peng Liu Cong‐Ying Zhou Song Xiang Chi‐Ming Che

Abstract An efficient silica‐supported iron terpyridine complex for oxidative C—C cross coupling reactions of tertiary amines with various carbon nucleophiles is described.

Terpyridine

Carbon fibers

10.1002/chin.201036148

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Practical iron-catalyzed atom/group transfer and insertion reactions

Pure and Applied Chemistry (2012)

Toby Wai‐Shan Chow Guo‐Qiang Chen Yungen Liu Cong‐Ying Zhou Chi‐Ming Che

Iron-catalyzed reactions are receiving a surge of interest owing to the natural abundance and biocompatibility of Fe and the urge to develop practically useful sustainable catalysis for fine chemical industries. This article is a brief account of our studies on the C–O and C–N bond formation reactions catalyzed by Fe complexes supported by oligopyridine, macrocyclic tetraaza, and fluorinated porphyrin ligands. The working principle is the in situ generation of reactive Fe=O and Fe=NR intermediates supported by these oxidatively robust N-donor ligands for oxygen atom/nitrogen group transfer and insertion reactions. The catalytic reactions include C–H bond oxidation of saturated hydrocarbons (up to 87 % yield), epoxidation of alkenes (up to 96 % yield), cis -dihydroxylation of alkenes (up to 99 % yield), epoxidation–isomerization (E–I) reaction of aryl alkenes (up to 94 % yield), amination of C–H bonds (up to 95 % yield), aziridination of alkenes (up to 95 % yield), sulfimidation of sulfides (up to 96 % yield), and amide formation from aldehydes (up to 89 % yield). Many of these catalytic reactions feature high regio- and diastereoselectivity and/or high product yields and substrate conversions, and recyclability of the catalyst, demonstrating the applicability of Fe-catalyzed oxidative organic transformation reactions in practical organic synthesis.

Amide

Dihydroxylation

10.1351/pac-con-11-11-08

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Citations (40)

Iron- and cobalt-catalyzed C(sp³)–H bond functionalization reactions and their application in organic synthesis

Chemical Society Reviews (2020)

Yungen Liu Tingjie You Haixu Wang Zhou Tang Cong‐Ying Zhou

This review highlights the developments in iron and cobalt catalyzed C(sp³)–H bond functionalization reactions with emphasis on their applications in organic synthesis, i.e. natural products and pharmaceuticals synthesis and/or modification.

Surface Modification

Organic Synthesis

10.1039/d0cs00340a

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Citations (158)

CCDC 1513962: Experimental Crystal Structure Determination

The Cambridge Structural Database (2019)

Jinhu Wei Bei Cao Chun‐Wai Tse Xiaoyong Chang Cong‐Ying Zhou

10.5517/ccdc.csd.cc1mtdhb

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Citations (0)