Discontinuous metal–insulator multilayers (DMIMs) of [CoFe( t n )/Al 2 O 3 ] m containing soft ferromagnetic (FM) Co 80 Fe 20 nanoparticles embedded discontinuously in a diamagnetic insulating Al 2 O 3 matrix are ideal systems to study interparticle interaction effects. Here the CoFe nanoparticles are treated as superspins with random size, position and anisotropy. At low particle density, namely nominal layer thickness t n = 0.5 nm, single-particle blocking phenomena are observed due to the absence of large enough interparticle interactions. However at 0.5 nm < t n < 1.1 nm, the particles encounter strong interactions which give rise to a superspin glass (SSG) phase. The SSG phase has been characterized by memory effect, ageing, dynamic scaling, etc. With further increase in particle concentration (1.1 nm < t n < 1.4 nm) and, hence, smaller interparticle distances, strong interactions lead to a FM-like state which is called superferromagnetic (SFM). The SFM state has been characterized by several techniques, e.g. dynamic hysteresis, Cole–Cole plots extracted from ac susceptibility, polarized neutron reflectometry, etc. Moreover, the SFM domains could be imaged by x-ray photoemission electron microscopy and magneto-optic Kerr effect microscopy. At t n > 1.4 nm physical percolation occurs between the particles and the samples are no longer discontinuous and then termed as metal insulating multilayers. Competition between long- and short-ranged dipolar interactions leads to an oscillating magnetization depth profile from CoFe layer to CoFe layer with an incommensurate periodicity.
Combined field- and current-induced domain wall (DW) motion in Permalloy microwires is studied using fast magneto-optical Kerr-microscopy. On increasing the current density, we find a decrease of Kerr signal contrast, corresponding to a reduction in the magnetization, which is attributed to Joule heating of the sample. Resistance measurements on samples with varying substrates confirm that the Curie temperature is reached when the magneto-optical contrast vanishes and reveal the importance of the heat flow into the substrate. By tuning the laser power, DWs can be pinned in the laser spot, which can thus act as a flexible pinning site for DW devices.
We study thermally assisted domain wall (DW) generation in perpendicular magnetic anisotropy CoFeB trilayer nanowires by the effect of Joule heating. The anomalous Hall effect is utilized to detect magnetization reversal in order to study the DW generation. We observe a statistical distribution in the switching process which is consistent with the thermal activation process. Our results show that the proposed method provides an efficient way for generating DWs in perpendicular magnetic nanowires at predefined locations.
We use a pump-probe photoemission electron microscopy technique to image the displacement of vortex cores in Permalloy discs due to the spin-torque effect during current pulse injection. Exploiting the distinctly different symmetries of the spin torques and the Oersted-field torque with respect to the vortex spin structure we determine the torques unambiguously, and we quantify the amplitude of the strongly debated nonadiabatic spin torque. The nonadiabaticity parameter is found to be β=0.15±0.07, which is more than an order of magnitude larger than the damping constant α, pointing to strong nonadiabatic transport across the high magnetization gradient vortex spin structures.
Magnetic resonance force microscopy (MRFM) is a scanning probe technique capable of detecting MRI signals from nanoscale sample volumes, providing a paradigm-changing potential for structural biology and medical research. Thus far, however, experiments have not reached suffcient spatial resolution for retrieving meaningful structural information from samples. In this work, we report MRFM imaging scans demonstrating a resolution of 0.9 nm and a localization precision of 0.6 nm in one dimension. Our progress is enabled by an improved spin excitation protocol furnishing us with sharp spatial control on the MRFM imaging slice, combined with overall advances in instrument stability. From a modeling of the slice function, we expect that our arrangement supports spatial resolutions down to 0.3 nm given suffcient signal-to-noise ratio. Our experiment demonstrates the feasibility of sub-nanometer MRI and realizes an important milestone towards the three-dimensional imaging of macromolecular structures.
Domain wall (DW) depinning and motion in the viscous regime induced by magnetic fields, are investigated in planar permalloy nanowires in which the Gilbert damping $\ensuremath{\alpha}$ is tuned in the range 0.008--0.26 by doping with Ho. Real time, spatially resolved magneto-optic Kerr effect measurements yield depinning field distributions and DW mobilities. Depinning occurs at discrete values of the field which are correlated with different metastable DW states and changed by the doping. For $\ensuremath{\alpha}<0.033$, the DW mobilities are smaller than expected while for $\ensuremath{\alpha}\ensuremath{\ge}0.033$, there is agreement between the measured DW mobilities and those predicted by the standard one-dimensional model of field-induced DW motion. Micromagnetic simulations indicate that this is because as $\ensuremath{\alpha}$ increases, the DW spin structure becomes increasingly rigid. Only when the damping is large can the DW be approximated as a pointlike quasiparticle that exhibits the simple translational motion predicted in the viscous regime. When the damping is small, the DW spin structure undergoes periodic distortions that lead to a velocity reduction. We therefore show that Ho doping of permalloy nanowires enables engineering of the DW depinning and mobility, as well as the extent of the viscous regime.
Magnetic sensing and logic devices based on the motion of magnetic domain walls rely on the precise and deterministic control of the position and the velocity of individual magnetic domain walls. Varying domain wall velocities have been predicted to result from intrinsic effects such as oscillating domain wall spin structure transformations and extrinsic pinning due to imperfections. We use direct dynamic imaging of the nanoscale spin structure to directly check these predictions. We find a new regime of oscillating domain wall motion even below the Walker breakdown correlated with periodic spin structure changes and we show that the extrinsic pinning from defects in the nanowire only affects slow domain walls.
We determine experimentally the spin structure of half-metallic Co2FeAl0.4Si0.6 Heusler alloy elements using magnetic microscopy. Following magnetic saturation, the dominant magnetic states consist of quasi-uniform configurations, where a strong influence from the magnetocrystalline anisotropy is visible. Heating experiments show the stability of the spin configuration of domain walls in confined geometries up to 800 K. The switching temperature for the transition from transverse to vortex walls in ring elements is found to increase with ring width, an effect attributed to structural changes and consequent changes in magnetic anisotropy, which start to occur in the narrower elements at lower temperatures.
Scanning magnetometry with nitrogen-vacancy (NV) centers in diamond has led to significant advances in the sensitive imaging of magnetic systems. The spatial resolution of the technique, however, remains limited to tens to hundreds of nanometers, even for probes where NV centers are engineered within 10 nm from the tip apex. Here, we present a correlated investigation of the crucial parameters that determine the spatial resolution: the mechanical and magnetic stand-off distances, as well as the subsurface NV center depth in diamond. We study their contributions using mechanical approach curves, photoluminescence measurements, magnetometry scans, and nuclear magnetic resonance (NMR) spectroscopy of surface adsorbates. We first show that the stand-off distance is mainly limited by features on the surface of the diamond tip, hindering mechanical access. Next, we demonstrate that frequency-modulated (FM) atomic force microscopy feedback partially overcomes this issue, leading to closer and more consistent magnetic stand-off distances (26–87 nm) compared with the more common amplitude-modulated feedback (43–128 nm). FM operation thus permits improved magnetic imaging of sub-100-nm spin textures, shown for the spin cycloid in BiFeO3 and domain walls in a CoFeB synthetic antiferromagnet. Finally, by examining 1H and 19F NMR signals in soft contact with a polytetrafluoroethylene surface, we demonstrate a minimum NV-to-sample distance of 7.9 ± 0.4 nm.
In a combined theoretical and experimental study, we investigate the critical current densities for vortex domain walls in magnetic nanowires. We systematically determine the critical current densities for continuous motion of vortex walls as a function of the wire width for different wire thicknesses and we find that the critical current density increases monotonously with decreasing wire width. Theoretically we present a mechanism that predicts a threshold current density based on wall transformations and this leads to a scaling of the critical current density ${j}_{c}\ensuremath{\propto}1/\text{width}$. The origin of this scaling is found to be the different dependence of the spin torque energy and the vortex nucleation energy on the wire width and good agreement with the experimental observations is found.
